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Ellingham Diagram

Ellingham Diagram for Ore Reduction · Also known as: Gibbs Free Energy Diagram, High-Temperature Reduction Diagram

The Ellingham Diagram, introduced by Harold Ellingham in 1944, is a graphical representation of the Gibbs free energy change for oxide formation and reduction as a function of temperature. It is an essential tool for predicting the thermodynamic feasibility of ore reduction and selecting appropriate reducing agents and temperatures for smelting and roasting operations.

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Ellingham Diagram
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When to use it

Use Ellingham diagrams when designing new smelting or roasting processes, evaluating ore feasibility, or troubleshooting existing operations. Assume equilibrium and ideal behavior. Kinetics and side reactions must be considered separately. Most valuable for screening alternatives before detailed thermodynamic or experimental studies.

Strengths & limitations

Strengths
  • Visual comparison of multiple reactions and temperatures on a single plot
  • Rapidly identifies thermodynamically favorable conditions without calculation
  • Guides selection of reducing agent (CO, H2, metal, etc.) and temperature
  • Shows where phase changes (melting) occur and their effect on ΔG°
  • Widely used in metallurgical education and industry; standard reference tool
Limitations
  • Assumes thermodynamic equilibrium; kinetics (reaction rate) are not shown
  • Does not account for side reactions or impurity effects unless explicitly plotted
  • Data are often for ideal conditions; real ore and slags deviate
  • Extrapolation beyond measured temperature ranges is unreliable
  • Multiple simultaneous reactions (e.g., sulfide roasting) require separate analysis

Frequently asked

How do I read an Ellingham diagram?

The y-axis is ΔG° (usually in kJ/mol of O2). The x-axis is temperature. Lines represent different oxide-formation reactions. Below a line, the oxide is stable. Above a line, the oxide reduces. Intersecting lines mark transition temperatures where one reducing agent becomes superior to another.

What if thermodynamics says reduction is unfavorable?

The reaction is thermodynamically impossible at that temperature and pressure. Increase temperature or change reducing agent. Alternatively, consider alternative process routes (e.g., sulfate leaching instead of direct reduction).

How do side reactions appear on Ellingham diagrams?

Side reactions are separate lines. If they are thermodynamically more favorable (lower ΔG°) than the desired reaction, they will compete. A good diagram shows all relevant competing reactions.

Do I need to achieve thermodynamic equilibrium?

Rarely. Smelters operate kinetically: they try to drive reactions fast enough, not necessarily to equilibrium. Kinetics (which Ellingham diagrams don't show) often limit conversion. Pilot testing is needed to confirm practical feasibility.

Where do I get accurate thermodynamic data for my ore?

Published databases (NIST, FactSage, HSC Chemistry) contain standard thermodynamic data. For non-standard ores, conduct differential scanning calorimetry (DSC) or thermogravimetric analysis (TGA) experiments to measure ΔH° and ΔS°.

Sources

  1. Ellingham, H. J. T. (1944). Reducibility of oxides and sulfides. Journal of the Society of Chemical Industry, 63(5), 125-160. link ↗
  2. Richardson, F. D. (2007). Physical chemistry of melts in metallurgy (Vol. 2). Academic Press. link ↗

How to cite this page

ScholarGate. (2026, June 3). Ellingham Diagram for Ore Reduction. ScholarGate. https://scholargate.app/en/mining-engineering/ellingham-diagram

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Referenced by

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CALPHADSlag BasicityMcCabe-Thiele MethodRedox Reaction Mechanism AnalysisElectrowinningShrinking Core ModelCyclic VoltammetryRDE Koutecky-Levich

Related reference concepts

Chemical ThermodynamicsElectrochemical ThermodynamicsPhase Diagrams and TransformationsChemical Potential and EquilibriumAqueous CorrosionPhase Equilibria and the Phase Rule

Spotted an issue on this page? Report or suggest a fix →

ScholarGate — Ellingham Diagram (Ellingham Diagram for Ore Reduction). Retrieved 2026-07-21 from https://scholargate.app/en/mining-engineering/ellingham-diagram · Dataset: https://doi.org/10.5281/zenodo.20539026
Quick facts
Originator
Harold Jeffrey Torreyson Ellingham
Subfamily
Thermodynamic Phase Diagrams
Year
1944
Type
Gibbs free energy diagram for high-temperature reactions
Related methods
ElectrowinningShrinking Core ModelSlag Basicity
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